Graphene makes ultrafast laser

Researchers at the University of Cambridge in the UK and CNRS in Grenoble, France, have fabricated an ultrafast "mode-locked" graphene laser. The result – which comes as quite a surprise, given the absence of a band gap in graphene – paves the way to photonic devices based on the material.

Since its discovery in 2004, graphene has continued to amaze scientists thanks to its unique electronic and mechanical properties that make it useful for a host of device applications. The "wonder material", as it is called, might even replace silicon as the electronic material of choice in the future. Graphene consists of a planar single sheet of carbon arranged in a honeycombed lattice and electrons travel through the material at extremely high speeds thanks to the fact that they behave like relativistic, or "Dirac", particles with no rest mass.

Now, Andrea Ferrari and colleagues say that graphene might be used in optoelectronics applications too, by demonstrating an ultrafast laser made from the material.

Ultrafast lasers are widely used in science and technology, and there is an increasing demand for compact, tunable laser sources. Today, the dominating technology in so-called mode-locked lasers – that is, lasers that produce ultrashort pulses at a very high repetition rate – is based on semiconductor saturable absorber mirrors (SESAMs). However, such devices are complicated and expensive to make, and are severely limited in their bandwidth.

Graphene mode-lockers

The new ultrafast laser exploits graphene and graphene layers as mode-lockers.

"In principle, this is quite a surprising result because graphene has no band gap, which is a key requirement for mode-locking in SESAMs," said Ferrari.

The team studied how light is absorbed in graphene and how photo-excited charge carriers behave in the material. In particular, they highlighted the key role of "Pauli blocking" in saturating the light absorption. Because of the Pauli exclusion principle, when pumping of electrons in the excited state is quicker than the rate at which they relax, the absorption saturates. This is because no more electrons can be excited until there is "space" available for them in the excited state.

Since the Dirac electrons in graphene linearly disperse, this means that it is the most wideband saturable light absorber ever, far out-passing the bandwidth provided by any other known material.

The researchers made their laser by starting with a graphene-polymer composite, obtained from a solution of graphene. Next, they placed this composite between two optical fibres in a laser cavity.

"Graphene is the ideal wideband saturable absorber, able to operate from the UV to visible and far-infrared wavelengths," Ferrari told our sister website nanotechweb.org. "Our graphene-based ultrafast laser, which harnesses the wideband optical nonlinearity of graphene, with no need for band gap engineering, extends the practical application of this novel material from nanoelectronics to optoelectronics and integrated photonics."

The team are now in the process of optimizing a fully functioning wideband tunable laser based on graphene, as well as trying similar experiments with graphene oxide.

The work was reported in ACS Nano.

Disk Laser Technology

A disk laser or active mirror is a type of solid-state laser characterized by a heat sink and laser output that are realized on opposite sides of a thin layer of active gain medium. It was introduced in the 1990s by the group of Adolf Giesen at the University of Stuttgart, Germany.

The gain medium of a thin-disk laser is a laser crystal (often Yb:YAG) in the form of a disk with a thickness of 100-200 µm, which is fixed on a water-cooled heat sink. The cooled end face has a dielectric coating that reflects both the laser radiation and the pump radiation.

The heat is extracted dominantly through the cooled end face, and because the disk thickness is considerably smaller than the laser beam diameter, the heat flow is largely in the direction of the beam, rather than in a transverse direction, as for a laser rod. As a consequence, thermal lensing is weak. The figure 1 illustrates the difference between the two types. Hence, the beam quality achievable with Disk Lasers can be much higher than that of a rod system, improving the Beam Parameter Product (BPP) up to 6 times.

The small disk thickness, as required to limit the heating, leads to incomplete pump absorption in a double pass. Therefore, one usually uses some multipass pumping scheme, which can be realized with very compact optics.

Due to improvements in the area of semiconductor pumping diodes the potential of Disk Lasers is not exhausted. While the first generation "only" extracted 1kW of laser power out of one disk, today's generation already generates 2kW out of one disk crystal. Still, the potential for this technology is not limited and expected to increase to 4kW per disk towards the end of 2008. Further, by combining several individual disk cavities, as illustrated in Figure 2, the total available laser power of a Disk Laser is virtually unlimited. The pumping beam from diode pumping stacks is reflected multi-fold via mirrors inside the cavity to pass up to 20 times through the disk. The disk "converts" the optical pumping light into a laser beam for processing. Based on an existing 4-cavity design, a laser power of 16kW will soon be available. The beauty of this Disk Laser principle over the fiber laser principle is that there are no losses in beam quality when scaling up laser power. These improvements in beam quality and power also lead to significant advantages for the design of processing optics and allowed the development of high-power scanner optics.

It is hardly necessary to mention that indispensable features known from conventional lamp-pumped lasers have not changed: Disk Lasers offer closed-loop power control, are insensitive against back reflections returning from the workpiece, their availability (uptime) is greater than 99 per cent and due to their modular construction all components can be replaced and maintained in the field. Last, but not least, for users of Disk Laser this means that not only the performance of such devices improves, but prices for say a 4 kW Disk Laser are falling because less cavities are required to generate the same laser power.

Q switching is possible with high pulse energies but not with very short pulses because the laser gain is quite limited.

Two Photon Absorption

The amount of light absorbed by a substance under normal single photon conditions is given by Beer’s Law, in which the amount of absorbed light is (in the weak absorption limit) proportional to the absorption cross-section of the molecule, s, the pathlength, l, and the concentration of absorbing species, C. In Two Photon Absorption (2PA), the absorption is proportional to the square of the light intensity. As a consequence, 2PA occurs only for very intense light, which, in common application, occurs at the focus of a laser beam. The photo at right shows fluorescence of a dye following 1PA and 2PA. The laser at the top of the cuvette is exciting the dye by 1PA causing yellow fluorescence emission. The emission can be seen clearly along the whole focussed laser path. The laser at the bottom of the cuvette is exciting the dye by 2PA, which causes the same yellow fluorescence. This time emission only occurs at the focal point of the laser because of the (intensity)2 dependence of the 2PA.

Simulated effects of excitation wavelength and numerical aperture on the dimensions of the 2PA volume. a, Normalized distributions of laser intensity-squared in the x-y and x-z plane for three different numerical apertures of water-immersion objective lenses at an excitation wavelength of 850 nm. Intensities-squared at lateral (x,y,0) and axial (x,0,z) positions were calculated using an ellipsoidal Gaussian approximation to the diffraction limited focus7,11 and expressed as the fraction of the intensity-squared at the focal point [I(0,0,0)2=1]. Color-coded contour plots depict isointensity lines in the x-z and x-y plane at the levels of 0.1, 0.3, 0.5, 0.7, and 0.9 of I(0,0,0)2. Note different scales for each panel. b, Dependence of 2PA volume on numerical aperture of the objective lens and illumination wavelength. Values were obtained by approximating the intensity-squared distribution as a three-dimensional Gaussian volume.12 For all calculations, it is assumed that the objective lens is uniformly illuminated (overfilled) and that no saturation of the fluorescence excitation process occurs. NA indicates numerical aperture.

Figure right provides a simplified illustration of the difference between single photon and two-photon activated processing. A material is polymerized along the trace of the moving laser focus, thus enabling fabrication of any desired polymeric 3D pattern by direct “recording” into the volume of photosensitive material. In a subsequent processing step the material, which was not exposed to the laser radiation, and therefore, stayed unpolymerized, is removed and the fabricated structure is revealed. The material sensitive in the UV range (λUV) can be polymerized by irradiation with the infra-red light of approximately double wavelength (λIR=2λUV), under the condition that the intensity of the radiation is high enough to initiate two-photon absorption.

First Pump-Probe Experiment at Linac Coherent Light Source Completed

(PhysOrg.com) -- The first experiment using the Linac Coherent Light Source to illuminate molecules via a "pump-probe" technique has been completed by an international team of more than 30 scientists from institutions including Lawrence Berkeley National Laboratory, LCLS and the joint SLAC/Stanford PULSE Institute. Ryan Coffee, physicist with the LCLS Laser Group, presented initial results in a seminar at SLAC on Wednesday, November 18.

Pump-probe experiments use one laser pulse, in this case an infrared pulse, to pump energy into a sample and then probe it with another laser pulse, in this case an LCLS X-ray pulse. Such experiments are ideal for looking at atomic and molecular interactions, which take place in tiny fractions of a second. The LCLS probe pulses were as short as a few quadrillionths of a second and a billion times brighter than any X-ray source produced in a laboratory.
Coffee and his colleagues looked at the quantum behavior of electrons in nitrogen molecules, N2. The results represent a step toward a fundamental understanding of how nature converts light into chemical energy and might one day help revolutionize solar power, Coffee said.
Nitrogen atoms distribute their electrons between a lower and a higher energy shell. Using X-rays, the team picked off two electrons from the lower level, allowing a higher shell electron to descend and fill the vacancy. The energy released during this downward plunge ejected another electron from the atom, a phenomenon known as the Auger effect.
The team wanted to study how the nitrogen molecules' orientation affected this reaction. To do this, they used the infrared laser to line up the nitrogen molecules so that they were all facing the same direction.
"In a sense, we tried to make the gas act a little bit like a crystal," Coffee said.
After hitting the nitrogen with X-rays, the researchers detected electrons flying off and measured how the molecules' alignment with respect to the X-rays influenced the Auger effect. They observed numerous features that had strong dependence on the molecules’ direction. The results are currently being prepared for publication.
Future work will focus on how atomic bonds change as molecules either break apart or rearrange. Coffee thinks such work will lead to a deeper understanding of how nature converts light into energy. Ultimately, he hopes the results will lead to technology that will help humans generate power from the sun.
"I'm going for the solar power revolution, though I don't know where it will come from," he said. His gut feeling is that the important atoms to look at are carbon, nitrogen and oxygen.
"That's where energy in nature comes from," he said.
Coffee added that the team owes a debt of gratitude to the LCLS Controls, Accelerator, and Laser Groups, who made the experiment's success possible.

Laser creates record-breaking protons

An international group of physicists working at the Los Alamos Laboratory in the US has used a laser to generate 67.5 MeV protons – the highest-energy protons yet produced in this way. Their work points the way to new laser-based devices for proton therapy, which would be far smaller and cheaper than existing particle-accelerator sources.

When a high-energy proton beam travels through the human body it deposits most of its energy within a small volume, the size and location of which can be calculated to great precision. As a result, protons offer a distinct advantage over other forms of radiation used to destroy tumour cells because they cause less damage to surrounding healthy tissue. Unfortunately, the accelerators needed to generate the protons can cover thousands of square metres and cost some $100m. This has limited the number of proton-therapy facilities available and patients often have to travel considerable distances to be treated in this way.

Some physicists believe that a laser-based proton generator could be made for about one tenth of the cost of a conventional accelerator and be small enough to be contained within a classroom-sized laboratory. The idea is that ultra-powerful laser pulses knock electrons out of the atoms within a tiny target, causing the electrons to accumulate on the target's rear surface. This sets up an electric field across the target, accelerating the resultant ions and forcing them to leave the material as a very high-energy beam.

Energy is a problem

In practice, however, some of the world's most powerful petawatt (10^15 W) lasers have only been able to generate protons with a maximum energy of about 58 megaelectronvolts (MeV). While tumours of the eye can be treated using protons of 60–70 MeV, deeper tumours require energies of about 300 MeV.

The latest breakthrough was carried out by Kirk Flippo of Los Alamos, Sandrine Gaillard of the Forschungszentrum Dresden–Rossendorf research centre (FZD) in Germany and colleagues, who used Los Alamos' Trident laser to generate 67.5 MeV protons. The work relies on a novel target design – an anvil-shaped piece of copper comprising a cone around 100 µm long with a 100 µm flat disc across perched on its tip. Flippo's team directed the laser beam to the inside of the cone, liberating electrons that were guided to the tip and which set up an electric field that accelerated protons away from the disc. The researchers claim that this arrangement is far more efficient than the thin films used in previous experiments – they used 80 J laser pulses, whereas the previous record of 58 MeV involved 450 J laser pulses.

Team-member Michael Bussmann of the FZD says that this significant step forward in maximum proton energy was also made possible by increasing the intensity of the main part of each pulse relative to the "pre-pulse", which precedes the main pulse and can damage the target.

Not enough protons

However, it might take a decade or more before laser-generated protons can be used to combat cancer. Another major challenge is that Trident and the other more intense lasers simply require too much energy to be able to function at the roughly 10 Hz pulse rate needed to produce enough protons for cancer therapy.

According to Bussmann, reaching the sought-after high production rates will be a matter of getting the target right. One possibility will be some kind of refinement of the anvil shape, he says. Others, however, believe that the answer lies in reducing the size of the target, allowing electrons to be heated and ejected from the target much more quickly and therefore with a more uniform energy distribution, in other words leading to fewer low-energy electrons. "We already have enough energy in our lasers, the question is how can we use it more efficiently," says Bussmann. "Nobody has the final idea right now," he said, "but we are in a position to test all these different theories and see which works best."

Looking beyond cancer therapy, Flippo believes that such proton sources could also be used to create medical isotopes and employed to generate neutrons for research in condensed-matter physics and other areas of science. They might also be used to search for nuclear materials inside cargo, given that the characteristics of a proton beam are altered in a well defined way by radioactive substances.

The research was presented at the annual meeting of the Division of Plasma Physics of the American Physical Society, held in Atlanta on 2–6 November.

Electron self-injection into an evolving plasma bubble

Just five years ago, experimentalists finally demonstrated that such laser-plasma accelerators could produce monoenergetic, collimated electron beams with quality comparable to conventional accelerators. The secret was for the laser to produce a "bubble" almost completely devoid of electrons in its immediate wake that captured electrons from the surrounding plasma and accelerated them in an exceptionally uniform way. Yet the precise mechanism by which the bubble captured these electrons and accelerated them with such uniformity has remained one of the outstanding mysteries of this field.

Now new theoretical work by scientists from the University of Texas and Commissariat à l'Énergie Atomique (CEA, France), to be reported at the 2009 APS Division of Plasma Physics Annual Meeting, has shed light on this mystery. Formation of the exceptional quality electron beam is attributed to the evolution of the bubble shape which, in turn, is directly associated with the nonlinear evolution of the driving laser pulse (nonlinear focusing and defocusing).

The basic premise of this work is that the size of the bubble—the cavity of electron density traveling over the positive ion background with nearly the speed of light—is determined by the spot size of the driving laser pulse. Plasma nonlinearities cause the laser to focus and defocus in the course of propagation. Once the laser diffracts, the bubble expands. Electrons that constitute a dense electron shell surrounding the bubble move with relativistic speeds and thus have high inertia. As a consequence, some of them become too heavy to follow the expanding shell; they fall inside the bubble, stay inside till the end of the plasma (i.e. get trapped) and finally gain multi-GeV energy.

The trapped charge is proportional to the bubble growth rate. Once the laser becomes self-guided, and the spot size oscillations saturate, the injection process clamps. Simultaneously, longitudinal non-uniformity of the accelerating gradient equalizes the trapped electron energy. This scenario of self-injection and monoenergetic bunch formation is discovered and explored in fine detail in the 3-D particle-in-cell simulations. This is fundamentally different from the previous work which concentrated on either one-dimensional models of electron trapping or on the reduced description of transverse plasma wave breaking in planar 2-D geometry.

The discussed mechanism of electron self-injection is very robust in experiments with the high-power laser (tens of terawatts to petawatt). In addition, an appropriate modification of the plasma density (e.g. using a thin dense slab as a nonlinear lens for the laser) may cause the laser to self-focus and defocus faster, which results in a single self-injection event. This kind of laser beam manipulation may lead to the generation of a 2.5 GeV mono-energetic (~1% energy spread) electron bunch containing ~1010 electrons in a future experiment with the recently commissioned Texas Petawatt (TPW) laser - the most powerful laser in the world. Electrons with 2.5 GeV of energy are traveling at 99.999998% of the speed of light. Electron beams with such unique properties are clearly beneficial for medical applications, radiation physics, material science, and homeland security.
Source: American Physical Society

Laser recreates X-rays emitted by a black hole

Physicists have used high-power lasers to recreate X-ray spectra emanating from some black holes and neutron stars. Conclusions drawn from the experiment appear to conflict with previous interpretations of astronomical data, suggesting that we may have to rethink our view of the structure surrounding black holes and neutrons stars.

Large quantities of X-rays are produced when a black hole or neutron star sucks in matter from a companion star, creating a ring of matter known as an accretion disc. As matter spirals into the black hole or neutron star, gravitational energy is converted into kinetic energy and heat. The intense radiation that is released travels outwards (in the form of photons) and ionizes material closer to the outer edge of the accretion disc – creating an X-ray emitting plasma.

Interpreting the X-ray spectrum of such a plasma is key to understanding the physics of such systems, because it is impossible for astronomers to directly measure its temperature, density and pressure. It has also proven very difficult to recreate such a "photo-ionized" plasma here on Earth because it requires an extremely hot source of radiation.

But now researchers in Japan, Korea and China are helping to address this weakness by studying the spectra of plasmas created in the lab. Such spectra are very similar to that produced by Cygnus X-3, a black hole and a companion star with highly ionized silicon ions on its surface. A similar X-ray spectrum has also been recorded from Vela X-1, a neutron-star binary system.

The researchers produced their X-ray spectra at the GEKKO-XII laser facility, which is located at Osaka University, Japan. The system combines a 10 TW laser that is capable of producing nanosecond pulses from twelve beams with a 10 PW laser that can deliver four picosecond beams.

"We used 12 nanosecond laser beams with wavelength, energy and pulse duration of 0.53 µm, 4 kJ in total and 1.2 ns [respectively]," explained Shinsuke Fujioka from Osaka University, who proposed and organized the experiment.

The beams are fired at a tiny plastic capsule, causing it to implode. "As it shrinks, a hot and dense plasma core forms inside the capsule," says Fujioka. The radiation produced then photo-ionizes a nearby sample of cold silicon gas.

Fujioka says that the shape of their X-ray spectra is quite similar to that recorded by astronomers. However, interpretations of the origin of characteristic lines emissions differ.

Astrophysicists claim that an X-ray peak at 1.84 keV stems from a forbidden transition of silicon ions. But Fujioka says that calculations performed by his team – which consider experimental measurements of the temperature and density of the plasma – suggest that the peak is associated with a different resonance transition of silicon ions. However, the researchers admit that they cannot provide a definite explanation for the origin of this peak. That is because the radiation flux produced in the laboratory lasts for tiny fractions of a second, while that produced by compact astrophysical objects is continuous.

The work is reported in Nature Physics and, writing in a companion piece, Paul Drake of the University of Michigan described the technique as having "great potential for further development," because it allows the energy of the photon source to be varied over a wide range while allowing a great deal of control over the photo-ionized material. However, Drake also cautions that more work must be done in terms of characterizing the physical properties of the resulting plasmas.

Fujioka says that the team may now turn its attention to investigations of the absorption of intense beams of X-rays. It is widely believed that the X-ray absorption rate in materials and plasmas is independent of the intensity of the beam, but they suspect that a plasma may become transparent in incredibly intense X-ray beams. If this is the case, it will modify our understanding of how plasmas behave in supernovae.

Airborne laser ready for flight tests

IT SHOULD be the moment of truth for the Airborne Laser (ABL). In the coming months, the multibillion-dollar laser built into a customised Boeing 747 will try to shoot a ballistic missile as it rises above the clouds.

Don't expect instant reports of success, though. Instead, if all goes to plan, we're likely to hear about a series of incremental improvements.

Developed by the US Department of Defense's Missile Defense Agency (MDA), the ABL aims to focus a beam of laser energy in the megawatt range for several seconds onto a missile at a "militarily significant distance" - more than 100 kilometres.

So far, the laser has only operated at near full power on the ground. On 18 August it was fired successfully from the air, but at reduced power. That, however, was no mean feat: aircraft vibrations play havoc with the precisely aligned optical components needed to generate a laser beam.

Firing at full power poses other challenges too. At powers high enough to destroy missiles, any surface contamination or tiny flaw in the laser optics can absorb so much heat that they crack or shatter.

High-power laser beams also heat the air they pass through, creating perturbations that can disperse or divert the beam. To counteract those effects, the ABL uses an adaptive system that senses atmospheric changes along its path and makes optical adjustments to compensate.

To test that system, the MDA plans a series of increasingly powerful shots at modified ballistic missiles loaded with sensors to measure the distribution of laser power on the target. Engineers will assess each shot's performance and use the results to fine-tune the adaptive optics. Once this is done, the MDA will test the laser again in varying conditions, and attempt to destroy actual missiles. The first of these tests is planned to take place late this year, with two more to follow in early 2010, according to an MDA spokeswoman.

A sister project, the Advanced Tactical Laser, which aims to use an airborne high-powered laser to hit targets on the ground, recently completed its first successful test. With future funding dependent upon the success of these tests, the pressure is on the ABL team to prove its efficacy.

Lasers Generate Sound in H2O

A new technology that uses flashes of laser light to remotely create underwater acoustics is being developed by scientists at the Naval Research Laboratory. The new acoustic source has the potential to expand and improve both Naval and commercial underwater acoustic applications, including undersea communications, navigation and acoustic imaging.

Dr. Ted Jones, a physicist in the Plasma Physics Division, is leading a team of researchers from the Plasma Physics, Acoustics, and Marine Geosciences Divisions in developing this acoustic source.

Efficient conversion of light into sound can be achieved by concentrating the light sufficiently to ionize a small amount of water, which then absorbs laser energy and superheats. The result is a small explosion of steam, which can generate a 220 decibel pulse of sound. Optical properties of water can be manipulated with very intense laser light to act like a focusing lens, allowing nonlinear self-focusing (NSF) to take place.

In addition, the slightly different colors of the laser, which travel at different speeds in water due to group velocity dispersion (GVD), can be arranged so that the pulse also compresses in time as it travels through water, further concentrating the light. By using a combination of GVD and NSF, controlled underwater compression of optical pulses can be attained.

The driving laser pulse has the ability to travel through both air and water, so that a compact laser on either an underwater or airborne platform can be used for remote acoustic generation. Since GVD and NSF effects are much stronger in water than air, a properly tailored laser has the ability to travel many hundreds of meters through air, remaining relatively unchanged, then quickly compress upon entry into the water. Atmospheric laser propagation is useful for applications where airborne lasers produce underwater acoustic signals without any required hardware in the water, such as undersea communications from aircraft.

Also, commercially available, high-repetition-rate pulsed lasers, steered by a rapidly movable mirror, can generate arbitrary arrays of phased acoustic sources. On a compact underwater platform with an acoustic receiver, such a setup can rapidly generate oblique-angle acoustic scattering data, for imaging and identifying underwater objects. This would be a significant addition to traditional direct backscattering acoustic data.

For more information, visit: www.nrl.navy.mil

Laser pulses control single electrons in complex molecules

Physicists of the Max Planck Institute of Quantum Optics (MPQ) in Garching and chemists of the Ludwig-Maximilians-Universität (LMU) in Munich, Germany, succeeded for the first time to use light for controlling single, negatively charged elementary particles in a bunch of electrons. The scientists achieved a major milestone that they aimed for within the excellence cluster "Munich Center for Advanced Photonics" (MAP). They report their results in the journal Physical Review Letters.

Electrons are extremely fast moving particles. In atoms and molecules they move on attosecond timescales. An attosecond is only a billionth of a billionth of a second. With light pulses that last only a few femtoseconds down to attoseconds it is possible to achieve control over these particles and to interact with them on the timescale of their motion. These short light pulses exhibit strong electric and magnetic fields influencing the charged particles. A femtosecond lasts 1000 times longer than an attosecond. In molecules with only a single electron, such as the deuterium molecular ion, their control with such light pulses is relatively easy. This was demonstrated in 2006 by a team of physicists including Professor Marc Vrakking and Dr. Matthias Kling from AMOLF in Amsterdam and Professor Ferenc Krausz in Garching (MPQ).

Scientists led by the junior research group leader Dr. Matthias Kling (MPQ) in collaboration with Professor Marc Vrakking (AMOLF) and Professor Regina de Vivie-Riedle (LMU) have managed to control and monitor the outer electrons from the valence shell of the complex molecule carbon monoxide (CO) utilizing the electric field waveform of laser pulses. Carbon monoxide has 14 electrons. With increasing number of electrons in the molecule the control over single electrons becomes difficult as their states lie energetically very close to each other.

In their experiments the scientists used visible (740 nm) laser pulses with 4 femtoseconds duration. The control was experimentally determined via an asymmetric distribution of C+ and of O+ fragments after the breaking of the molecular bond. The measurement of C+ and O+ fragments implies a dynamic charge shift along the molecular axis in one or the other direction, controlled via the laser pulse.

The femtosecond laser pulses initially detached an electron from a CO molecule. Subsequently the electron was driven by the laser field away from and back to the ion, where it transferred its energy in a collision. The whole process took only ca. 1.7 femtoseconds. "The collision produces an electronic wave packet which induces a directional movement of electrons along the molecular axis," says Regina de Vivie-Riedle. "The excitation and subsequent interaction with the remainder of the intense laser pulse leads to a coupling of electron and nuclear motion and gives a contribution to the observed asymmetry," explains Matthias Kling.

The scientists could also image the structure and form of the outer two electron orbitals of carbon monoxide via the ionization process. The extremely short femtosecond laser pulses allowed the scientists to explore this process in the outermost orbitals. They found the ionization of the molecules to take place with a distinct angular dependence with respect to the laser polarization direction. This observation was found to be in good agreement with theoretical calculations and also gave a contribution to the observed asymmetry. The scientists could show that the strength of this asymmetry strongly depends on the duration of the laser pulses.

With their experiments and calculations, the researchers from Garching and Munich have achieved an important milestone that they aimed for within the excellence cluster "Munich Center for Advanced Photonics" (MAP). The goals were to achieve and observe the control of single electrons within a multi-electron system.

Electrons are present in all important microscopic biological and technical processes. Their extremely fast motion on the attosecond timescale, determines biological and chemical processes and also the speed of microprocessors - technology at the heart of computing. With their experiments the researchers have made a further, important step towards the control of chemical reactions with light. The results are also related to basic research on lightwave electronics aiming at computing speeds on attosecond timescales.

More information: Znakovskaya, P. von den Hoff, S. Zherebtsov, A. Wirth, O. Herrwerth, M.J.J. Vrakking, R. de Vivie-Riedle, M.F. Kling: “Attosecond control of electron dynamics in carbon monoxide”, Physical Review Letters (4. September 2009)

New study will contribute to better understanding of nuclear ignition

UCSD scientists create computer simulations like the ones above to determine how to successfully achieve controlled, miniaturized nuclear ignition of spherical fuel pellets in laboratory environments using lasers as energy drivers.

Under a recent three-year, $510,000 grant from the National Nuclear Security Administration (NNSA), Vu and his colleagues at Los Alamos National Laboratory (NM), Lodestar Research Corporation and the Laboratory for Laser Energetics at the University of Rochester in New York, are using computer simulation tools to figure out how to successfully achieve controlled, miniaturized nuclear ignition of spherical fuel pellets in laboratory environments using lasers as energy drivers.

Vu said the primary lasers for these studies are the Omega laser at the University of Rochester (NY) and the newly built National Ignition Facility at Lawrence Livermore National Laboratory (CA).

"What we would like to do is take the laser and shine the laser onto what we call a hohlraum, a cylindrically shaped black-body radiator made of high-Z materials (typically gold), in the middle of which the miniaturized fuel pellet is placed," he explained. "The material on the wall of the hohlraum absorbs the laser energy, heats up, and becomes a plasma. The plasma in turn irradiates off its newly acquired energy, and the resulting black-body radiation is what drives the miniaturized fuel pellets to nuclear ignition. It's like sunlight hitting the dashboard of a car - the energy of the sunlight is absorbed by the dashboard and is irradiated as heat, essentially electromagnetic radiation on a different wavelength spectrum from the original sunlight. It's a lot of fancy physics. But if you think about in on a fundamental level, it's pretty simple.

Source: University of California - San Diego

Transparent aluminium is 'new state of matter'

(PhysOrg.com) -- Oxford scientists have created a transparent form of aluminium by bombarding the metal with the world’s most powerful soft X-ray laser. 'Transparent aluminium' previously only existed in science fiction, featuring in the movie Star Trek IV, but the real material is an exotic new state of matter with implications for planetary science and nuclear fusion.

In this week’s Nature Physics an international team, led by Oxford University scientists, report that a short pulse from the FLASH laser ‘knocked out’ a core electron from every aluminium atom in a sample without disrupting the metal’s crystalline structure. This turned the aluminium nearly invisible to extreme ultraviolet radiation.

''What we have created is a completely new state of matter nobody has seen before,’ said Professor Justin Wark of Oxford University’s Department of Physics, one of the authors of the paper. ‘Transparent aluminium is just the start. The physical properties of the matter we are creating are relevant to the conditions inside large planets, and we also hope that by studying it we can gain a greater understanding of what is going on during the creation of 'miniature stars' created by high-power laser implosions, which may one day allow the power of nuclear fusion to be harnessed here on Earth.’

The discovery was made possible with the development of a new source of radiation that is ten billion times brighter than any synchrotron in the world (such as the UK’s Diamond Light Source). The FLASH laser, based in Hamburg, Germany, produces extremely brief pulses of soft X-ray light, each of which is more powerful than the output of a power plant that provides electricity to a whole city.

The Oxford team, along with their international colleagues, focused all this power down into a spot with a diameter less than a twentieth of the width of a human hair. At such high intensities the aluminium turned transparent.

Whilst the invisible effect lasted for only an extremely brief period - an estimated 40 femtoseconds - it demonstrates that such an exotic state of matter can be created using very high power X-ray sources.

Professor Wark added: ‘What is particularly remarkable about our experiment is that we have turned ordinary aluminium into this exotic new material in a single step by using this very powerful laser. For a brief period the sample looks and behaves in every way like a new form of matter. In certain respects, the way it reacts is as though we had changed every aluminium atom into silicon: it’s almost as surprising as finding that you can turn lead into gold with light!’

The researchers believe that the new approach is an ideal way to create and study such exotic states of matter and will lead to further work relevant to areas as diverse as planetary science, astrophysics and nuclear fusion power.

A report of the research, 'Turning solid aluminium transparent by intense soft X-ray photoionization', is published in Nature Physics. The research was carried out by an international team led by Oxford University scientists Professor Justin Wark, Dr Bob Nagler, Dr Gianluca Gregori, William Murphy, Sam Vinko and Thomas Whitcher.

Military mega-lasers are too hot to handle

HIGH-ENERGY laser weapons have been hailed as the future of anti-missile defence, but they may be further from being battle-ready than military chiefs hoped.

In recent tests, several prototypes have suffered serious damage to their optics at intensities well below the expected levels of tolerance. "Optical damage has been quietly alarming upper management in most major programmes," Sean Ross of the US Air Force Research Laboratory in New Mexico told a meeting of the Directed Energy Professional Society in Newton, Massachusetts, last week. There are also big problems managing the waste heat generated by high-intensity beams.

Laser weapons require mirrors and lenses to focus powerful beams onto distant moving targets, and to compensate for atmospheric perturbations that can reduce the power they deliver. The higher the intensity of the beam, the more likely it is to damage the surface of its optical components.

Optical surfaces are designed to withstand powers up to a specific damage threshold, but tiny flaws or irregularities - which can be extremely difficult to spot - reduce this threshold by making them more vulnerable to heat. Contaminants deposited on the surface can also reduce this threshold by forcing the surface to absorb energy.

These problems have begun to stall the development of laser weapons. Earlier this year in the US, engineers halted tests of the $4.3 billion megawatt-class Airborne Laser short of full power to avoid damaging "a handful of optics in the turret", according to Mike Rinn, a Boeing vice-president who manages the programme. They realised that the optics, designed years ago, would be "frail" in the presence of any contamination, which would be virtually inevitable in flight. In the next week or so, Boeing engineers will install replacement optics and test them on the ground before running the laser at full power in flight.

Finding a way of preventing laser weapons from frying themselves is proving just as troublesome. Depending on the type of laser, generating 1 watt of laser beam produces about 4 watts of waste heat that must be dissipated. The challenge is to develop a cooling system that is both small and extremely robust.

Laser-created temporal lens could lead to movies of molecular processes

(PhysOrg.com) -- Finding a way to observe and record the behavior of matter at the molecular level has long been a holy grail among physicists. That ability could open the door to a wide range of applications in ultrafast electron microscopy used in a large array of scientific, medical and technological fields.

Now, a team at the University of Nebraska-Lincoln has figured out a possible way to do that. Working in collaboration with Nobel laureate Ahmed Zewail (chemistry, 1999) of the California Institute of Technology in Pasadena, they developed mathematical models to show that laser beams create ultra-high-speed "temporal lenses" that would be capable of making "movies" of molecular processes. The finding was published in the June 15-19 online edition of the Proceedings of the National Academy of Sciences.

The "lenses" in question are not made of glass like those found in standard tabletop microscopes. They're created by laser beams that would keep pulses of electrons from dispersing and instead focus the electron packets on a target. The timescales required, however, are hardly imaginable on a human scale -- measured in femtoseconds (quadrillionths of a second) and attoseconds (quintillionths of a second).

The physicists modeled two types of lenses. One was a temporal "thin" lens created using one laser beam that could compress electron pulses to less than 10 femtoseconds. The second was a "thick" lens created using two counterpropagating laser beams that showed the potential of compressing electron pulses to reach focuses of attosecond duration.

Europe's big lasers: the exawatt roadmap

Europe is thinking big – big lasers, big science, big budgets. Over the next decade, a trio of planned pan-European research facilities will give scientists access to unprecedented laser powers and intensities, opening the door to exotic science that will shed light on the origins of the universe and, it is hoped, provide the foundations for a sustainable energy future.

The overall construction cost for this new generation of "super lasers" is in excess of €2 bn, with operational budgets running to several hundred million euros per year. That's a price worth paying, says Christian Kurrer, research programme officer at the European Commission.

"International infrastructures attract the best research scientists," Kurrer told delegates attending the "Emerging European Laser Facilities: Beyond Petawatt" workshop at the recent SPIE Europe conference in Prague, Czech Republic. "The infrastructures are well beyond the man-power and financial resources on a national level. This is why we need more collaborative efforts."

One of those collaborations is the High Power Laser Energy Research (HiPER) facility. Headed up by the UK Science and Technology Facilities Council (STFC), a research funding body, HiPER's mission is to carry out proof-of-principle research into energy generation from laser-driven inertial-confinement fusion. The grand challenge: to initiate and study nuclear-fusion reactions via laser heating of a millimetre-sized fuel pellet (containing a mixture of deuterium and tritium) to temperatures greater than 100 million °C.

Although construction of HiPER is not slated to begin until 2014, the process of whipping existing laser technology into shape to deliver a light source with the requisite capabilities is already under way. "Current laser capability has reached its culmination in the petawatt (10^15 W) scale," observed Mike Dunne, project director of HiPER and a senior scientist at the Rutherford Appleton Laboratory (RAL), UK. "We're looking at how to take it [the technology] to the next generation."

This is the purpose of the three-year preparatory phase on HiPER, which is running alongside initial experiments at the US Department of Energy's $4 bn (€3.1 bn) National Ignition Facility (NIF) in California. (As with HiPER, the end-game for NIF, a huge facility consisting of 192 pulsed laser beams with a total energy of 1.8 MJ, is the creation of nuclear fusion in the laboratory.)

Another major European laser facility in the works is the Extreme Light Infrastructure (ELI), a project that's being led by scientists at the Laboratoire d'Optique Appliquée (LOA) at the Ecole Polytechnique, Palaiseau, France. Scheduled to fire up in 2015, ELI will enable fundamental science to be carried out at the very highest laser powers (in the exawatt regime, 10^18 W) and intensities (10^24 W/cm2).

Like HiPER, ELI will allow academic researchers to explore fundamental science at the extremes (stuff like photon–photon scattering and other nonlinear quantum vacuum effects). Other missions outlined in the ELI project include attosecond science (e.g. the study of the ultrafast motion of electrons inside atoms over timescales of the order of 10^–18 s) and generating a secondary source of electron beamlines from the light-matter interaction. HiPER, meanwhile, will also enable scientists to study laser–plasma interactions and "laboratory astrophysics" (e.g. the creation of conditions in the lab that could yield insights into supernovae evolution).

The European X-ray Free Electron Laser (European XFEL) is dedicated to generating ultrashort, hard X-ray flashes for a range of basic and applied research, including atomic-scale metrology and time-resolved studies of chemical reactions down to the 100 fs regime. Construction began on the 3.4 km long laser facility at DESY, an established particle physics and photonics research laboratory in Hamburg, Germany, at the beginning of the year.

DESY has taken the technology and knowhow from an existing pilot facility, FLASH, which is optimized for the extreme UV and soft X-ray range. "The European XFEL is based on the knowledge that has been accumulated at FLASH," said Tschentscher. "DESY will continue to operate FLASH as a user facility for the 6–60 nm regime and the European XFEL will basically build a new machine covering the wavelength range from below 0.1 nm up to 6 nm."

Upon completion, the European XFEL is intended to provide the brightest source of hard X-ray pulses at the highest repetition rate (30,000 flashes per second). In an initial version electron bunches will be separated into three beamlines delivering coherent pulses to six different experimental stations tuned to specific wavelengths.

• This article originally appeared in the June 2009 issue of Optics & Laser Europe magazine.

Study gives clues to increasing X-rays' power

In a paper to be published in an upcoming edition of Physical Review Letters, UNL Physics and Astronomy Professor Anthony Starace and his colleagues give scientists important clues into how to unleash coherent, high-powered X-rays.

"This could be a contributor to a number of innovations," Starace said.

Starace's work focuses on a process called high-harmonic generation, or HHG. X-ray radiation can be created by focusing an optical laser into atoms of gaseous elements - usually low-electron types such as hydrogen, helium, or neon. HHG is the process that creates the energetic X-rays when the laser light interacts with those atoms' electrons, causing the electrons to vibrate rapidly and emit X-rays.

But the problem with HHG has been around almost as long as the onset of the method in 1988: The X-ray light produced by the atoms is very weak. In an effort to make the X-rays more powerful, scientists have attempted using higher-powered lasers on the electrons, but success has been limited.

"Using longer wavelength lasers is another way to increase the energy output of the atoms," Starace said. "The problem is, the intensity of the radiation (the atoms) produce drops very quickly."

Instead of focusing on low-electron atoms like hydrogen and helium, Starace's group applied HHG theory to heavier (and more rare) gaseous atoms having many electrons - elements such as xenon, argon and krypton. They discovered that the process would unleash high-energy X-rays with relatively high intensity by using longer wavelength lasers (with wavelengths within certain atom-specific ranges) that happen to drive collective electron oscillations of the many-electron atoms.

"If you use these rare gases and shine a laser in on them, they'll emit X-Rays with an intensity that is much, much stronger (than with the simple atoms)," Starace said. "The atomic structure matters."

Starace said that unlocking the high-powered X-rays could lead one day, for example, to more powerful and precise X-ray machines. For instance, he said, heart doctors might conduct an exam by scanning a patient and creating a 3D hologram of his or her heart, beating in real time.

Nanoscientists, who study the control of matter on an atomic or molecular scale, also may benefit from this finding, Starace said. Someday, the high-intensity X-rays may be used to make 3D images of the microscopic structures with which nanoscientists work.

"With nanotechnology, miniaturization is the order of the day," he said. "But nanoscientists obviously could make use of a method to make the structures they're building and working with more easily visible."

Big lasers, big science, big questions

Leading optical scientists agree that research and industry stakeholders need to do more if Europe is to maximize the benefits from a planned new generation of high-power laser facilities. That was one of the headline messages from the "Emerging European Laser Facilities: Beyond Petawatt" workshop at the SPIE Europe conference in Prague, Czech Republic, last week.

Marking 50 years since the invention of the laser, the workshop was intended to open debate among senior figures from planned pan-European petawatt laser facilties (1015 W and beyond). Among the "blue-ribbon" initiatives under discussion were projects like HiPER (the High Power Laser Energy Research project), ELI (the Extreme Light Infrastructure), and the European X-Ray Laser project (XFEL).

"International infrastructures attract the best research scientists," Christian Kurrer, research programme officer at the European Commission, told delegates. "The infrastructures are well beyond the man-power and financial resources on a national level. This is why we need more collaborative efforts."

With access to unprecedented laser power and scientific expertise, it is easy to see why large-scale science facilities are attractive to users. In fact, some might argue that they are too good and that they will pull in users (and resources) simply because they can guarantee results where smaller national institutions can't. "Industries want facilities for reproducible, reliable results and 100% service," was the opinion of Mike Dunne, HiPER project director.

At the same time, workshop participants agreed that there's plenty of work to do to ensure that stakeholders in research and industry are in position to maximize their interactions with "big science". "They [the laser facilities] have the scientific experts and we bring the industrial methods where the networks can really make a difference," said Federico Canova of Amplitude Technologies, a French laser manufacturer.

New European Union member states might also question the economic returns on their investment in big science, not least because the planned locations for all of these big laser facilities are in western Europe. Kurrer, however, prefers to view such challenges as opportunities. "While distribution [of projects] may never be good, the key will be to break down the borders. Europe is all about talking to each other and overcoming barriers."

Europe's new generation of high-energy laser facilities form part of an ambitious big-science roadmap coordinated by the European Strategy Forum on Research Infrastructures (ESFRI). The ESFRI roadmap covers capital and operational investments running to tens of billions of euros in strategic research areas like energy, environmental science and advanced materials.

Shaking the Fundamentals of Physics: At the Limits of the Photoelectric Effect

By way of the classical photoeffect, Einstein proved in 1905 that light also has particle character. However, with extremely high light intensities, remarkable things happen in the process. Scientists of the Physikalisch-Technische Bundesanstalt (Germany) have found this out with colleagues at FLASH in Hamburg, the first free-electron laser (FEL) for soft X-rays worldwide.

The current models based on Einstein's idea are simply described in such a way: A photon knocks an external electron out of an atom, provided that the photon energy is high enough. However, with wavelengths of only 13 nanometers and high radiation intensities of several petawatt per square centimeter something else - at least with some atoms - happens: With xenon, a whole light-wave packet immediately seems to knock out a huge number of internal electrons. This effect is strongly dependent on the material and not only on the characteristics of the exciting radiation, as accepted before. The work, which is currently published in the journal Physical Review Letters, has significance for future experiments of materials research at the new large X-ray laser facilities of the world.

The scientists actually wanted to develop methods for the radiometric characterization of X-ray lasers. They irradiated different gases to derive the laser strength from the ionization effect. The aim: with the laser well characterized was, for example, the testing of EUV lithography mirrors. The EUV lithography (EUV stands for extreme ultraviolet) at wavelengths in the range of 13 nanometers is considered as the future technology for the production of ever smaller computer chips.

However, during their experiments at FLASH, the new free-electron laser (FEL) in Hamburg, which currently allows the generation of EUV radiation and soft X-rays of the highest intensity in the world, they unexpectedly discovered things which concern the fundamentals of physics.

With the classical photoelectric effect (a), a single light particle (photon) of sufficient energy interacts with a single electron of the material. The process is energetically described by the Einstein equation (1905) and demonstrates the quantum structure of light. Only at very high intensities, does the multiphoton ionization occur, a process which is described in the extreme case of highly intensive ultra-short light flashes as emitted by long-wave femtosecond lasers, again, in the wave picture of light (b).

Nevertheless, the suitable theoretical models fail in the short-wave X-ray regime as shown by the experiments in Hamburg in which, for the first time, soft X-ray irradiance levels of several petawatts per square centimeter were achieved by strong beam focusing. The comparative quantitative studies prove that the degree of light-matter interaction and, thereby, the nature of the X-ray light are decisively determined by the structure of the atom and correlations in, above all, inner electron shells.

In the extreme case (xenon), a whole wave packet of photons seems to lead to the simultaneous emission of several inner electrons (c).

More information: Extreme ultraviolet laser excites atomic giant resonance. M. Richter et al., Phys. Rev. Lett. (2009) - online publication expected: April 27, 2009.

Photoelectric effect at ultra-high intensities. A. A. Sorokin et al., Phys. Rev. Lett. 99, 213002 (2007)

Source: Physikalisch-Technische Bundesanstalt

Curved light bends the rules

Everyone knows that light travels in a straight line — right? A couple of years back, however, physicists discovered something very different for certain laser pulses that have one intense peak next to a series of smaller peaks. The brightest part of these lopsided "Airy" pulses, they found, appear to follow a curved trajectory.

Researchers in the US have now found that sufficiently intense Airy pulses can ionize the surrounding air molecules and create curved filaments of plasma. What's more, Airy pulses interact with air such that the pulses are continually focused and so can travel long distances without being dispersed.

The bright white light given off by the plasma filaments could be used make remote spectroscopic measurements of the atmosphere — and the bending effect itself could be exploited in new kinds of waveguide.

The bendy behaviour of Airy pulses was first discovered in 2007 by Demetrios Christodoulides and colleagues at the University of Florida. Interference between the peaks causes the intense peak to veer off in one direction, while the other peaks move in the opposite direction. Although the total momentum of the pulse travels in a straight line, its brightest part appears to follow a curved path.

Christodoulides and his colleagues have now teamed up with Pavel Polynkin and others at the University of Arizona to create curved “filaments” of plasma using Airy pulses. The key to their success, according to Jerome Kasparian of the University of Geneva who was not part of the group, is their ability to — for the first time — create Airy pulses of extremely high intensity.

The team began with an intense infrared laser pulse that is about 35 fs in duration. The initially pancake-shaped pulse, which is symmetric around its direction of propagation, is then passed through a “phase mask” and then a lens, giving it a chevron shape with an intense peak at the vertex (see figure). This Airy pulse then travels about 1 m through air to a fluorescent screen where the light is detected.

As well as confirming that extremely intense Airy pulses appear to curve, the pulses also produced curved filaments of plasma by ionizing nearby molecules in the air.

Although physicists have long known that symmetric laser pulses can create such filaments, the process has proved very difficult to study. This is because symmetric laser pulses travel in the same direction as the white light given off by the plasmas they create, which means that any device that attempts to detect this light is dazzled or even destroyed by the pulse.

With Airy pulses, however, Polynkin, Christodoulides and colleagues discovered that the plasma light travels in straight lines tangentially to the curvature of the bright peak. The plasma light can therefore be detected — and perhaps even be used as a source of white light for spectroscopy.

Firing intense and long-range pulses into the air, for example, could allow researchers to make remote spectroscopic measurements of the atmosphere.

Polynkin also speculates that intense pulses could be fired into thunderclouds to create filaments that "guide" lightning to safe locations on the ground.

Studying the plasma light itself could even help physicists gain a better understanding of the complicated non-linear optics that define how intense laser beams travel through air. These include a “self-healing” effect whereby the beam is continually refocused by the plasma — rather than being dispersed — allowing intense pulses to travel very long distances.

The team are now studying the creation of curved filaments in water rather than air.

Soliton laser offers broad tunability

A femtosecond soliton source with fast and broad spectral tunability has been developed by researchers in Argentina. The source, which comprises a Ti:sapphire laser and a highly nonlinear photonic-crystal fibre, can be tuned from 850 nm to 1000 nm with nearly constant pulse width and average power (Optics Letters 34 842).

The key to the laser's tuning performance is the use of solitons generated in the photonic-crystal fibre. At the low-power coupling regime, solitons can be tuned over a broad range of wavelengths from 850 to 1000 nm. The solitons generated in the fibre maintain almost constant pulse and spectral widths regardless of input power.

In the set-up, a photonic-crystal fibre measuring 75 cm in length is pumped with a Ti:sapphire laser that provides 37 fs pulses at a repetition rate of 94 MHz and a wavelength of 830 nm. Average power ranging from 1 to 10 mW is pumped into the fibre, controlled by an acousto-optic modulator (AOM).