Materials can be grouped in three categories according to their electric properties: metals provide free charge carriers, i.e. electrons, under any conditions, and therefore conduct electricity when exposed to even small electric fields. In semiconductors, on the other hand, the charge carriers require a certain 'energy kick' before they are able to move around. This is why semiconductors are very well suited as the basic material for electronic switching components in which the digits "0" and "1" are represented by an "on" or "off" current, respectively. The best silicon-based semiconductor components available today allow switching between these two states several billion times per second, i.e. at gigahertz-rates (1 GHz = 109 Hz). This corresponds to the frequency of microwaves.
The third group of materials are so-called dielectrics. Here, the electrons are more or less immobile, therefore, dielectrics are insulators under normal conditions; at very low electric fields they don't conduct electric current, whereas at high static fields they suffer irreversible damage. The team of Prof. Krausz now took interest in the question of how such materials would respond to very high and (usually) destructive fields that act on it for just a tiny moment. To this way they used a special tool: very short and intensive laser pulses of visible/near-infrared light with a duration of a few femtoseconds (1 fs is a millionth of a billionth of a second), which contain only a couple of cycles with a perfectly controlled waveform. In these pulses, the amplitude of the oscillating electric field increases from moderate values to more than 10 billion Volts per metre extremely rapidly, within a few femtoseconds.
In the first experiment [1] the scientists investigated whether these light pulses would cause dielectrics to conduct electric currents at all. Their test object was a small silica-glass prism, coated on two sides with gold electrodes with a 50 nanometre wide gap in between. After irradiating the prism with the intense few-femtosecond pulses, an electric current was measured between the electrodes. "Two effects are contributing to this result", Tim Paasch-Colberg explains, who worked on this experiment as a doctoral candidate. "On the one hand the strong electric field of one pulse enhances the mobility of the electrons. On the other hand, the appropriately directed weaker field of a second pulse pushes the mobilised electrons towards the gold electrodes." The experiments revealed that the electric current changes its direction as the weak (driving) field is delayed by half a wave period (about 1.2 fs) with respect to the strong (mobilizing) field. "This behaviour is a strong indication that the material is turned from an insulator into a conductor by the strong light field within less than a femtosecond," Tim Paasch-Colberg says. "However, from these observations we cannot yet conclude that the conductivity can also be switched off within the same time scale, which is a precondition for the effect being utilized for signal processing."
Attosecond real-time observation of changes in the electronic properties of a dielectric |
Both sets of experiments can be described with one and the same microscopic model developed by Vadym Apalkov and Mark Stockman, which explains – based on quantum mechanics – the underlying physical processes and supports the conclusion of full reversibility of the observed light-induced changes. "Our work demonstrates how state-of-the-art photonic techniques may explore ways of pushing the frontiers of information processing," says Agustin Schiffrin, leading the first project and currently researcher at the University of British Columbia (Vancouver, Canada). Professor Krausz, head of the Laboratory for Attosecond Physics, likes to put these measurements into a larger context: "We hope that these results provide motivation for other groups worldwide to join us in exploring and exploiting the potential wide-gap materials may offer for speeding up electronics."
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