Making sharper X-rays

A photograph of the custom-built laser chamber, which receives simultaneously a pulse of helium gas and a pulse from RIKEN’s free-electron laser, which is known as the SPring-8 Compact SASE Source (SCSS). The resulting blue-green superfluorescence is visible.

A variety of imaging technologies rely on light with short wavelengths because it allows very small structures to be resolved. However, light sources which produce short, extreme ultraviolet or x-ray wavelengths often have unstable emission wavelength and timing. Now, by illuminating a gas with a powerful laser, a research team in Japan has demonstrated a light source that may solve many of these problems. The research was published by Mitsuru Nagasono, from the RIKEN SPring-8 Center in Harima, and his colleagues from RIKEN and three other institutes.

More information: Nagasono, M., et al. Observation of free-electron-laser-induced collective spontaneous emission (superfluorescence). Physical Review Letters 107, 193603 (2011).

Plasmonics produces extreme UV light

An international team of researchers has invented a simple way of creating ultrashort pulses of extreme ultraviolet (EUV) light. The system uses a new 3D metallic waveguide, or "nanofunnel", that coverts pulses of infrared light to EUV.

EUV light has a wavelength of around 5–50 nm, which is about 100–10 times shorter than that of visible light. As a result, ultrashort pulses of EUV light are ideal for studying fundamental physics phenomena – such as how electrons move in atoms, molecules and solids.

However, it is difficult to produce EUV radiation using conventional methods that rely on using amplified light pulses from an oscillator (a source of laser light) to ionize noble gas atoms. The electrons liberated during this process are accelerated in the light field and their surplus energy is freed as attosecond (10–18 s) pulses of light of different wavelengths. The shortest wavelengths of light can then be "filtered out" to produce a single EUV pulse – a complicated process.
Simpler way of making pulses

Now, researchers at the Korea Advanced Institute of Science and Technology (KAIST), the Max Planck Institute of Quantum Optics (MPQ) in Germany and Georgia State University (GSU) in the US have come up with a different – and much simpler – way of doing things.

The new technique works by converting femtosecond (10–15 s) infrared pulses into femtosecond EUV pulses. The process exploits surface-plasmon polaritons (SPPs), which are particle-like collective oscillations that occur when light interacts with a metal's conduction electrons.

The nanofunnel made by the KAIST-MPQ-GSU team was devised so that it concentrated incident infrared light pulses into a spot that is smaller than the wavelength of the incident light. The funnel is a metallic nanostructure made of silver that contains a hollow hole shaped like a tapered cone. The cone is just a few micrometres long and filled with xenon gas. The tip of the funnel is around 100 nm across.

The researchers sent infrared light pulses (at a rate of 75 MHz) into the funnel, which is designed so that it contains patches of metal that are positively charged, followed by patches that are negatively charged. This arrangement produces electromagnetic fluctuations on the inside walls of the funnel, which result in the creation of SPPs. These particles then travel towards the tip, where the conical shape of the funnel concentrates their fields.

"The field on the inside of the funnel can become a few hundred times stronger than the field of the incident infrared light," explains Mark Stockman of GSU. "This enhanced field results in the generation of EUV light in the Xe gas."

An important feature of the nanofunnel is that it can be produced at frequencies of up to about 75 MHz. Seung-Woo Kim, team leader at KAIST, where the experiments were carried out, adds: "Due to their short wavelength and potentially short pulse duration, EUV light pulses can be an important tool for exploring electron dynamics in atoms, molecules and solids. Electrons move very fast – on the attosecond timescale – and light flashes that are shorter than attoseconds long are therefore needed to image these particles. Although scientists routinely use attosecond light flashes for such studies, they have much lower frequencies. Our new nanofunnel could change all this."

The results are detailed in Nature Photonics.

Shaking the Fundamentals of Physics: At the Limits of the Photoelectric Effect

By way of the classical photoeffect, Einstein proved in 1905 that light also has particle character. However, with extremely high light intensities, remarkable things happen in the process. Scientists of the Physikalisch-Technische Bundesanstalt (Germany) have found this out with colleagues at FLASH in Hamburg, the first free-electron laser (FEL) for soft X-rays worldwide.

The current models based on Einstein's idea are simply described in such a way: A photon knocks an external electron out of an atom, provided that the photon energy is high enough. However, with wavelengths of only 13 nanometers and high radiation intensities of several petawatt per square centimeter something else - at least with some atoms - happens: With xenon, a whole light-wave packet immediately seems to knock out a huge number of internal electrons. This effect is strongly dependent on the material and not only on the characteristics of the exciting radiation, as accepted before. The work, which is currently published in the journal Physical Review Letters, has significance for future experiments of materials research at the new large X-ray laser facilities of the world.

The scientists actually wanted to develop methods for the radiometric characterization of X-ray lasers. They irradiated different gases to derive the laser strength from the ionization effect. The aim: with the laser well characterized was, for example, the testing of EUV lithography mirrors. The EUV lithography (EUV stands for extreme ultraviolet) at wavelengths in the range of 13 nanometers is considered as the future technology for the production of ever smaller computer chips.

However, during their experiments at FLASH, the new free-electron laser (FEL) in Hamburg, which currently allows the generation of EUV radiation and soft X-rays of the highest intensity in the world, they unexpectedly discovered things which concern the fundamentals of physics.

With the classical photoelectric effect (a), a single light particle (photon) of sufficient energy interacts with a single electron of the material. The process is energetically described by the Einstein equation (1905) and demonstrates the quantum structure of light. Only at very high intensities, does the multiphoton ionization occur, a process which is described in the extreme case of highly intensive ultra-short light flashes as emitted by long-wave femtosecond lasers, again, in the wave picture of light (b).

Nevertheless, the suitable theoretical models fail in the short-wave X-ray regime as shown by the experiments in Hamburg in which, for the first time, soft X-ray irradiance levels of several petawatts per square centimeter were achieved by strong beam focusing. The comparative quantitative studies prove that the degree of light-matter interaction and, thereby, the nature of the X-ray light are decisively determined by the structure of the atom and correlations in, above all, inner electron shells.

In the extreme case (xenon), a whole wave packet of photons seems to lead to the simultaneous emission of several inner electrons (c).

More information: Extreme ultraviolet laser excites atomic giant resonance. M. Richter et al., Phys. Rev. Lett. (2009) - online publication expected: April 27, 2009.

Photoelectric effect at ultra-high intensities. A. A. Sorokin et al., Phys. Rev. Lett. 99, 213002 (2007)

Source: Physikalisch-Technische Bundesanstalt

Extreme UV light made easy

A new system to generate coherent extreme-ultraviolet (EUV) light has been developed by researchers in Korea. The device, based on a nanostructure made of bow-tie shaped gold "antennas" on a sapphire substrate, is smaller and cheaper than existing systems and might allow an EUV source the size of a laptop computer to be made. Potential applications for the source include high-resolution biological imaging, advanced lithography of nanoscale patterns and perhaps even "X-ray clocks".

EUV light has a wavelength of between around 5 and 50 nm (100–10 times shorter than that of visible light). It can thus be used to etch patterns at tiny length scales and is ideal for spectroscopic applications because the wavelength is the same as that of many atomic transitions.

However, EUV radiation is currently produced in a very complicated process involving the use of amplified light pulses from an oscillator (a source of laser light) to ionize noble gas atoms. The electrons freed during this process are accelerated in the light field and their surplus energy is freed as attosecond (10^–18 s) pulses of light of different wavelengths. The shortest wavelengths of light can then be "filtered out" to produce a single EUV pulse.

Scientists would ideally like to produce EUV light directly from the oscillator without the need for expensive and bulky amplifiers. In this way, EUV-light generation could be simplified and the size of the source significantly reduced to tabletop dimensions. In contrast, current devices usually measure around 2–3 m across. Now, Seung-Woo Kim of KAIST in Daejeon and colleagues have shown that this might be possible.

The researchers report that a bow-tie nanostructure of gold – measuring around 20 nm across – can enhance the intensity of femtosecond laser light pulses by two orders of magnitude. This is high enough to generate EUV light with a wavelength of less than 50 nm directly from a small pulse with an energy of 10^11 W/cm^2 injected into argon gas (Nature 453 757). The energy needed is about 100 times less than in traditional approaches.

Surface plasmons

The technique works thanks to "surface plasmons" (surface excitations that involve billions of electrons) in the "gap" of the bow-tie gold nanostructures (see figure). When illuminated with the correct frequency of laser light, the surface plasmons can begin to resonate in unison, greatly increasing the local light field intensity. This phenomenon, known as resonant plasmon field enhancement, is already exploited in imaging techniques, such as surface-enhanced Raman scattering, which is sensitive enough to detect individual molecules on a metal surface.

Immediate applications include high-resolution imaging of biological objects, advanced lithography of nanoscale patterns and making X-ray clocks. These exploit a frequency-stabilized femtosecond laser and are being investigated worldwide to replace the current caesium atomic clocks for better time precision.

"This new method of short-wavelength light generation will open doors in imaging, lithography and spectroscopy on the nanoscale," commented Mark Stockman of the Georgia State University in a related article (Nature 453 731). The spatially coherent, laser-like light could have applications in many areas: spectroscopy; screening for defects in materials; and, if extended to X-ray or gamma-wavelengths, detecting minute amounts of fissile materials for public security and defence.

The team now plans to improve the conversion efficiency of the generated light by modifying the design of their nanostructure – for example, by making 3D cones with sharper tips. These will not only enable higher local field enhancement but also better interaction of the femtosecond light pulses with injected gas atoms. The team will also test the spatial and temporal coherence of the generated EUV light.

Source: Physicsworld.com; Phtonics.com; Optics.org

Generation of intense continuum EUVradiation by many-cycle laser fields

The scientists at Institute of Electronic Structure & Laser in Greece and Max-Planck-Institut für Quantenoptik in Germany reported their research results in recent issue of Nature Physics.

Continuing efforts in ultrashort pulse engineering have recently led to the breakthroughs of the generation of attosecond (10^-18 s) pulse trains and isolated pulses. Although trains of multiple pulses can be generated through the interaction of many-optical-cycle pulses with gases—a process that has led to intense extreme-ultraviolet emission—the generation of isolated high-intensity pulses, which requires few-cycle driving pulses, remains a challenge. Here, we report a vital step towards the generation of such pulses, the production of broad continuum extreme-ultraviolet emission using a high-intensity, many-cycle, infrared pulsed laser, through the interferometric modulation of the ellipticity of 50-fs-long driving pulses. The increasing availability of high-power many-cycle lasers and their potential use in the construction of intense attosecond radiation—with either gas or solid-surface targets—offer exciting opportunities for multiphoton extreme-ultraviolet-pump–extreme-ultraviolet-probe studies of laser–matter and laser–plasma interactions.

The Dual Michelson interferometer device is shown in the left picture, BS: beam splitters. M: flat mirrors. TS1,2,3: piezoelectric translation stages. A: intensity attenuator. First and second MI: first and second Michelson interferometers.

Plasma mirrors generate high harmonics

For many researchers working with high-intensity lasers, plasma formation is often bad news. For others, it’s an enabling step for putting their laser systems to good use, in the form of so-called plasma mirrors. Now, collaborators at CEN Saclay (Gif-sur-Yvette, France), École Polytechnique (Palaiseau, France), and the University of Toronto (Toronto, Ont., Canada) have used a chain of plasma mirrors to create extreme-ultraviolet (EUV) pulses that they predict to be on the attosecond timescale, all with a tabletop laser.

In the highest intensity femtosecond-laser systems, a nanosecond-scale prepulse can be enough to ablate the surface of samples before most of the pulse energy arrives. Enter the plasma mirror, a simple but effective solution to increase the contrast between the prepulse and the main pulse. By placing a highly polished mirror blank in the beam at Brewster’s angle, the nanosecond-scale prepulse passes unchanged. The rising edge of the main pulse, however, converts the surface of the mirror into a highly reflective plasma, specularly reflecting only the main pulse. Once the prepulse is cleaned up by two plasma mirrors, a third forms the basis for high-order harmonic generation (HHG).

C. Thaury et al.,Nature Phys. doi:10.1038/nphys595 (2007).