KBBF crystal gives direct access to DUV

Researchers in China have created a tunable all-solid-state laser that emits milliwatt power levels in the deep ultraviolet (DUV). Applications requiring light around the 200 nm mark, such as photoemission spectroscopy and photolithography, could benefit from this work (Applied Physics B 93 323).

"Our source tunes from 175 to 210 nm via fourth harmonic generation from a Ti:sapphire laser," Zuyan Xu of the Chinese Academy of Sciences told optics.org. "The highest output power is 2.23 mW at 193 nm but the power is above 1 mW between 182 and 210 nm. This is the first demonstration of a milliwatt-level widely tunable all-solid-state laser below 200 nm by direct second harmonic generation."

The team's set-up can essentially be broken into three stages: the initial nanosecond-pulsed Ti:sapphire laser, optics to generate the second harmonic in the UV and additional components to generate the fourth harmonic in the DUV.

The output from the Ti:sapphire (more than 3W across the range of 690–840 nm) is focused into a set of BBO crystals to generate UV light between 340 and 415 nm. This light is then passed into the KBBF crystal to generate the DUV wavelengths.

When it comes to producing tunable DUV light, one alternative approach is sum-frequency mixing. This however uses two laser beams making the system complex and of limited practical use. To remove this complexity, Xu and colleagues use a KBBF crystal that offers a direct route to DUV light below 200 nm using just one beam.

Ultraviolet pulses close in on 1 fs regime

Deep ultraviolet (DUV) pulses with a duration of just 3.7 femtoseconds have been generated by researchers at the Max-Planck-Institute for Quantum Optics in Germany. The pulses are said to be the shortest ever observed at this wavelength range and could allow the team to influence the outcome of chemical reactions by controlling the motion of electrons in molecules. (Optics Express 16 18956)

Previously, the shortest pulses in the DUV (wavelengths shorter than 300 nm) had a duration of 8 femtoseconds. Much of the research effort focused on compressing the ultraviolet pulses after they had been generated, which is a formidable challenge as this requires precise dispersion control.

Here, Ulrich Graf and colleagues take a different approach. They upconvert 780 nm, 0.25 mJ pulses with a duration of 6 femtosecond pulses directly into the UV range by means of harmonic generation in a noble gas jet.

The resulting 3.7 femtosecond pulses are characterized using a dispersion-minimized SD-FROG approach and have energies in excess of 1.4µJ. The conversion efficiency is approximately 0.6%.

The group is now hoping to extend its approach to generate ultrashort pulses in the vacuum ultraviolet (VUV) spectral range (wavelengths less than 180 nm). "In the VUV, matter absorbs light even more and this spectral range will offer plenty of opportunities to explore and control the microcosm on an ultrafast scale," said Goulielmakis. "At the same time, we anticipate that these pulses will be substantially shorter and will approach the 1 femtosecond frontier."